I just did this, and decided on the 58 cc chambers. Most of my experience has been with 68 to 79 blocks. In spite of published numbers, both of my rebuilds calculated out to about 8.5 to barely 9.1 compression, due to the conservative nature of replacement pistons, and the deck height tolerance on the blocks. Even with the iron GT40 heads at 64 cc or less there just is not much compression.
So I decided that the smaller chambers would provide some compression, getting up to 9.2 or so.
If you are not going to add a blower, I would put as much compression in there as you can, up to 9.8 to 1 or so. If it detonates, you can reduce the timing for daily driving, and put better gas in when you want to hammer it.
For a NA car, I would go with the small chambers.